Abstract
We present a novel heterodyne-detected four-wave mixing technique, which determines the third-order nonlinear polarization in phase and amplitude by spectral interferometry. It allows us to measure the resonant transient four-wave mixing of single localized excitons, both frequency and time-resolved. In the signal, the strength of the coupling between two probed exciton transitions is directly observable. Applying a strong optical pump pulse, we observe optical Rabi oscillations of the exciton polarization. Observing decay of the third-order polarization after the pump pulse, we can exclude the presence of signi£cant excitation-induced dephasing.
| Language | English |
|---|---|
| Title of host publication | Physics of Semiconductors |
| Subtitle of host publication | 27th International Conference on the Physics of Semiconductors, ICPS-27 |
| Pages | 1232-1233 |
| Number of pages | 2 |
| Volume | 772 |
| DOIs | |
| Publication status | Published - 30 Jun 2005 |
| Event | PHYSICS OF SEMICONDUCTORS: 27th International Conference on the Physics of Semiconductors, ICPS-27 - Flagstaff, AZ, United States Duration: 26 Jul 2004 → 30 Jul 2004 |
Conference
| Conference | PHYSICS OF SEMICONDUCTORS: 27th International Conference on the Physics of Semiconductors, ICPS-27 |
|---|---|
| Country | United States |
| City | Flagstaff, AZ |
| Period | 26/07/04 → 30/07/04 |
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Keywords
- nanomaterials
- interferometry
- four wave mixing
- quantum information
- excitons
- quantum optics
Cite this
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Transient four-wave mixing of single exciton states : exciton-exciton interaction and Rabi oscillations. / Patton, B.; Langbein, W.; Woggon, U.
Physics of Semiconductors: 27th International Conference on the Physics of Semiconductors, ICPS-27. Vol. 772 2005. p. 1232-1233.Research output: Chapter in Book/Report/Conference proceeding › Conference contribution book
TY - GEN
T1 - Transient four-wave mixing of single exciton states
T2 - exciton-exciton interaction and Rabi oscillations
AU - Patton, B.
AU - Langbein, W.
AU - Woggon, U.
PY - 2005/6/30
Y1 - 2005/6/30
N2 - We present a novel heterodyne-detected four-wave mixing technique, which determines the third-order nonlinear polarization in phase and amplitude by spectral interferometry. It allows us to measure the resonant transient four-wave mixing of single localized excitons, both frequency and time-resolved. In the signal, the strength of the coupling between two probed exciton transitions is directly observable. Applying a strong optical pump pulse, we observe optical Rabi oscillations of the exciton polarization. Observing decay of the third-order polarization after the pump pulse, we can exclude the presence of signi£cant excitation-induced dephasing.
AB - We present a novel heterodyne-detected four-wave mixing technique, which determines the third-order nonlinear polarization in phase and amplitude by spectral interferometry. It allows us to measure the resonant transient four-wave mixing of single localized excitons, both frequency and time-resolved. In the signal, the strength of the coupling between two probed exciton transitions is directly observable. Applying a strong optical pump pulse, we observe optical Rabi oscillations of the exciton polarization. Observing decay of the third-order polarization after the pump pulse, we can exclude the presence of signi£cant excitation-induced dephasing.
KW - nanomaterials
KW - interferometry
KW - four wave mixing
KW - quantum information
KW - excitons
KW - quantum optics
U2 - 10.1063/1.1994558
DO - 10.1063/1.1994558
M3 - Conference contribution book
SN - 0735402574
SN - 9780735402577
VL - 772
SP - 1232
EP - 1233
BT - Physics of Semiconductors
ER -