Pump-power-dependence of CsPbBr3-in-Cs4PbBr6 quantum dot color converter

Miguel F. Leitão, Mohamed Sufyan Islim, L. Yin, S. Viola, S. Watson, A. Kelly, Y. Dong, X. Li, H. Zeng, S. Videv, H. Haas, E. Gu, I. M. Watson, N. Laurand, M. D. Dawson

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Abstract

The detailed study of the pump-intensity dependent characteristics of an all-inorganic CsPbBr3-in-Cs4PbBr6 quantum dot (QD) color converter is reported. This is an attractive material to color convert UV/blue GaN optical pump sources for digital lighting applications, e.g. visible light communications (VLC). It demonstrates narrow spectral emission (522 nm peak emission and < 20 nm full-width-at-half-maximum), invariant with the pump power density (from 0 to 7.15 kW/cm2). The optical bandwidth increases, from 10 MHz at 300 μW/cm2, up to 22 MHz at 3 W/cm2, and 41 MHz at 7.15 kW/cm2. This acceleration of the emission is ascribed to both an increase of the radiative decay rate in the low-pump-density regime, and to the emergence of non-radiative pathways at higher pump density. The higher bandwidth at high-pump density enables a 30% increase in the data rate of a free space VLC link using this color converter.
Original languageEnglish
Pages (from-to)3504-3518
Number of pages15
JournalOptical Materials Express
Volume9
Issue number8
Early online date29 Jul 2019
DOIs
Publication statusPublished - 1 Aug 2019

Keywords

  • quantum dot
  • colour converter
  • pump power density

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    CsPbBr3-in-Cs4PbBr6 quantum dot color converter

    Leitao, M. (Creator), Laurand, N. (Supervisor) & Dawson, M. (Supervisor), University of Strathclyde, 30 Jul 2019

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    Cite this

    Leitão, M. F., Islim, M. S., Yin, L., Viola, S., Watson, S., Kelly, A., Dong, Y., Li, X., Zeng, H., Videv, S., Haas, H., Gu, E., Watson, I. M., Laurand, N., & Dawson, M. D. (2019). Pump-power-dependence of CsPbBr3-in-Cs4PbBr6 quantum dot color converter. Optical Materials Express, 9(8), 3504-3518. https://doi.org/10.1364/OME.9.003504