Pulses of carbon dioxide emissions from intracrustal faults following climatic warming

Niko Kampman, Neil Burnside, Zoe K. Shipton, Hazel J. Chapman, Joe A. Nicholl, Rob M. Ellam, Mike J. Bickle

Research output: Contribution to journalArticle

71 Citations (Scopus)

Abstract

Carbon capture and geological storage represents a potential means of managing atmospheric carbon dioxide levels. Understanding the role of faults, as either barriers or conduits to the flow of carbon dioxide, is crucial for predicting the long-term integrity of geological storage sites. Of particular concern is the influence of geochemical reactions on the sealing behaviour of faults and the impact of seismicity and stress regime on fault stability. Here, we examine a 135,000-year palaeorecord of carbon dioxide leakage from a faulted, natural carbon dioxide reservoir in Utah. We assess the isotope and trace-element composition of U-Th-dated carbonate veins, deposited by carbon-dioxide-rich fluids. Temporal changes in vein geochemistry reveal pulses of carbon dioxide injection into the reservoir from deeper formations. Surface leakage rates increase by several orders of magnitude following these pulses. We show that each pulse occurs around 100-2,000 years after the onset of significant local climatic warming, at glacial to interglacial transitions. We suggest that carbon dioxide leakage rates increase as a result of fracture opening, potentially caused by changes in groundwater hydrology, the intermittent presence of a buoyant gas cap and postglacial crustal unloading of regions surrounding the fault.

Original languageEnglish
Pages (from-to)352–358
Number of pages7
JournalNature Geoscience
Volume5
Early online date22 Apr 2012
DOIs
Publication statusPublished - May 2012

Keywords

  • carbon dioxide
  • geological storage sites
  • carbon dioxide leakage
  • geochemistry
  • tectonics

Research Output

  • 71 Citations
  • 4 Article

Man-made versus natural CO2 leakage: a 400 k.y. history of an analogue for engineered geological storage of CO2

Burnside, N., Shipton, Z., Dockrill, B. & Ellam, R. M., Apr 2013, In : Geology. 41, 4, p. 471-474 4 p.

Research output: Contribution to journalArticle

65 Citations (Scopus)

Rapid river incision across an inactive fault—Implications for patterns of erosion and deformation in the central Colorado Plateau

Pederson, J., Burnside, N., Shipton, Z. & Rittenour, T., Oct 2013, In : Lithosphere. 5, 5, p. 513-520 8 p.

Research output: Contribution to journalArticle

  • 11 Citations (Scopus)

    He and Ne as tracers of natural CO2 migration up a fault from a deep reservoir

    Gilfillan, S. M. V., Wilkinson, M., Haszeldine, R. S., Shipton, Z. K., Nelson, S. T. & Poreda, R. J., Nov 2011, In : International Journal of Greenhouse Gas Control . 5, 6, p. 1507–1516 10 p.

    Research output: Contribution to journalArticle

  • 55 Citations (Scopus)

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