Operando neutron scattering – following reactions in real time using neutrons

Vainius Skukauskas; Elliot L.B. Johnson Humphrey; Iain Hitchcock; Andrew York; Joseph Kelleher; Emma K. Gibson; David J. Nelson; Ian P. Silverwood

doi:10.1007/s11244-021-01436-x

Operando neutron scattering – following reactions in real time using neutrons

Vainius Skukauskas, Elliot L.B. Johnson Humphrey, Iain Hitchcock, Andrew York, Joseph Kelleher, Emma K. Gibson, David J. Nelson, Ian P. Silverwood

Pure And Applied Chemistry

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Abstract

The complexation of NiCl2 with 2,2'-Bipyridine was followed using quasielastic neutron scattering to observe reaction progress. Water adsorption in chabazite with time resolution was observed using strain induced in the aluminosilicate framework with a high-resolution engineering diffractometer. These reactions illustrate the recent progress and possibilities in using neutron probes to observe realistic catalytic reactions as they progress.

Original language	English
Pages (from-to)	693-698
Number of pages	6
Journal	Topics in Catalysis
Volume	64
Issue number	9-12
DOIs	https://doi.org/10.1007/s11244-021-01436-x
Publication status	Published - 17 May 2021

Keywords

Operando
catalysis
neutron diffraction
quasielastic neutron scattering
QENS

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10.1007/s11244-021-01436-x

Skukauskas-etal-TIC-2021-Operando-neutron-scattering-following-reactions-in-real-time-using-neutronsAccepted author manuscript, 651 KB

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abstract = "The complexation of NiCl2 with 2,2'-Bipyridine was followed using quasielastic neutron scattering to observe reaction progress. Water adsorption in chabazite with time resolution was observed using strain induced in the aluminosilicate framework with a high-resolution engineering diffractometer. These reactions illustrate the recent progress and possibilities in using neutron probes to observe realistic catalytic reactions as they progress.",

keywords = "Operando, catalysis, neutron diffraction, quasielastic neutron scattering, QENS",

author = "Vainius Skukauskas and \{Johnson Humphrey\}, \{Elliot L.B.\} and Iain Hitchcock and Andrew York and Joseph Kelleher and Gibson, \{Emma K.\} and Nelson, \{David J.\} and Silverwood, \{Ian P.\}",

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doi = "10.1007/s11244-021-01436-x",

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AU - Skukauskas, Vainius

AU - Johnson Humphrey, Elliot L.B.

AU - Hitchcock, Iain

AU - York, Andrew

AU - Kelleher, Joseph

AU - Gibson, Emma K.

AU - Nelson, David J.

AU - Silverwood, Ian P.

PY - 2021/5/17

Y1 - 2021/5/17

N2 - The complexation of NiCl2 with 2,2'-Bipyridine was followed using quasielastic neutron scattering to observe reaction progress. Water adsorption in chabazite with time resolution was observed using strain induced in the aluminosilicate framework with a high-resolution engineering diffractometer. These reactions illustrate the recent progress and possibilities in using neutron probes to observe realistic catalytic reactions as they progress.

AB - The complexation of NiCl2 with 2,2'-Bipyridine was followed using quasielastic neutron scattering to observe reaction progress. Water adsorption in chabazite with time resolution was observed using strain induced in the aluminosilicate framework with a high-resolution engineering diffractometer. These reactions illustrate the recent progress and possibilities in using neutron probes to observe realistic catalytic reactions as they progress.

KW - Operando

KW - catalysis

KW - neutron diffraction

KW - quasielastic neutron scattering

KW - QENS

UR - https://www.springer.com/journal/11244

U2 - 10.1007/s11244-021-01436-x

DO - 10.1007/s11244-021-01436-x

M3 - Article

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EP - 698

JO - Topics in Catalysis

JF - Topics in Catalysis

IS - 9-12

ER -

Operando neutron scattering – following reactions in real time using neutrons

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Keywords

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