New evidence for the influence of step morphology on the formation of Au atomic chains on vicinal Si(111) surfaces

N. McAlinden, J. F. McGilp

Research output: Contribution to journalArticle

16 Citations (Scopus)

Abstract

Gold atomic chain structures that grow on singular and vicinal Si(111) surfaces have attracted considerable interest as model systems for exploring quasi-one-dimensional metallic behaviour. The structure of the prototypical Si(111)-5 x 2-Au system remains controversial, however. Reflection anisotropy spectroscopy provides new, independent evidence supporting a recently proposed three-Au-chain structure. For stepped surfaces, the results provide good evidence that a single Au chain forms adjacent to [(1) over bar(1) over bar2] steps and a double Au chain forms adjacent to [11 (2) over bar] steps. In both cases spectral lineshape and coverage data support a three-chain Si(111)-5 x 2-Au structure forming over the remainder of the terrace. For all the vicinal Si(111) surfaces, including Si(557) and Si(775), it is the step morphology, and not the terrace width, that determines whether single- or double-Au-chain structures are formed in the region of the steps.

Original languageEnglish
Article number67008
Pages (from-to)-
Number of pages5
JournalEPL: A Letters Journal Exploring the Frontiers of Physics
Volume92
Issue number6
DOIs
Publication statusPublished - 31 Dec 2010

Fingerprint

gold
anisotropy
spectroscopy

Keywords

  • SI surfaces
  • electromigration
  • anisotropy
  • silicon
  • gold

Cite this

@article{42e26a8e48af4d848bec6dbedca36563,
title = "New evidence for the influence of step morphology on the formation of Au atomic chains on vicinal Si(111) surfaces",
abstract = "Gold atomic chain structures that grow on singular and vicinal Si(111) surfaces have attracted considerable interest as model systems for exploring quasi-one-dimensional metallic behaviour. The structure of the prototypical Si(111)-5 x 2-Au system remains controversial, however. Reflection anisotropy spectroscopy provides new, independent evidence supporting a recently proposed three-Au-chain structure. For stepped surfaces, the results provide good evidence that a single Au chain forms adjacent to [(1) over bar(1) over bar2] steps and a double Au chain forms adjacent to [11 (2) over bar] steps. In both cases spectral lineshape and coverage data support a three-chain Si(111)-5 x 2-Au structure forming over the remainder of the terrace. For all the vicinal Si(111) surfaces, including Si(557) and Si(775), it is the step morphology, and not the terrace width, that determines whether single- or double-Au-chain structures are formed in the region of the steps.",
keywords = "SI surfaces, electromigration, anisotropy , silicon, gold",
author = "N. McAlinden and McGilp, {J. F.}",
year = "2010",
month = "12",
day = "31",
doi = "10.1209/0295-5075/92/67008",
language = "English",
volume = "92",
pages = "--",
journal = "EPL: A Letters Journal Exploring the Frontiers of Physics",
issn = "0295-5075",
number = "6",

}

TY - JOUR

T1 - New evidence for the influence of step morphology on the formation of Au atomic chains on vicinal Si(111) surfaces

AU - McAlinden, N.

AU - McGilp, J. F.

PY - 2010/12/31

Y1 - 2010/12/31

N2 - Gold atomic chain structures that grow on singular and vicinal Si(111) surfaces have attracted considerable interest as model systems for exploring quasi-one-dimensional metallic behaviour. The structure of the prototypical Si(111)-5 x 2-Au system remains controversial, however. Reflection anisotropy spectroscopy provides new, independent evidence supporting a recently proposed three-Au-chain structure. For stepped surfaces, the results provide good evidence that a single Au chain forms adjacent to [(1) over bar(1) over bar2] steps and a double Au chain forms adjacent to [11 (2) over bar] steps. In both cases spectral lineshape and coverage data support a three-chain Si(111)-5 x 2-Au structure forming over the remainder of the terrace. For all the vicinal Si(111) surfaces, including Si(557) and Si(775), it is the step morphology, and not the terrace width, that determines whether single- or double-Au-chain structures are formed in the region of the steps.

AB - Gold atomic chain structures that grow on singular and vicinal Si(111) surfaces have attracted considerable interest as model systems for exploring quasi-one-dimensional metallic behaviour. The structure of the prototypical Si(111)-5 x 2-Au system remains controversial, however. Reflection anisotropy spectroscopy provides new, independent evidence supporting a recently proposed three-Au-chain structure. For stepped surfaces, the results provide good evidence that a single Au chain forms adjacent to [(1) over bar(1) over bar2] steps and a double Au chain forms adjacent to [11 (2) over bar] steps. In both cases spectral lineshape and coverage data support a three-chain Si(111)-5 x 2-Au structure forming over the remainder of the terrace. For all the vicinal Si(111) surfaces, including Si(557) and Si(775), it is the step morphology, and not the terrace width, that determines whether single- or double-Au-chain structures are formed in the region of the steps.

KW - SI surfaces

KW - electromigration

KW - anisotropy

KW - silicon

KW - gold

U2 - 10.1209/0295-5075/92/67008

DO - 10.1209/0295-5075/92/67008

M3 - Article

VL - 92

SP - -

JO - EPL: A Letters Journal Exploring the Frontiers of Physics

JF - EPL: A Letters Journal Exploring the Frontiers of Physics

SN - 0295-5075

IS - 6

M1 - 67008

ER -