High performance vertical organic electrochemical transistors

Mary J. Donahue, Adam Williamson, Xenofon Strakosas, Jacob T. Friedlein, Robert R. McLeod, Helena Gleskova, George G. Malliaras

Research output: Contribution to journalArticle

8 Citations (Scopus)

Abstract

Organic electrochemical transistors (OECTs) are promising transducers for biointerfacing due to their high transconductance, biocompatibility, and availability in a variety of form factors. Most OECTs reported to date, however, utilize rather large channels, limiting the transistor performance and resulting in a low transistor density. This is typically a consequence of limitations associated with traditional fabrication methods and with 2D substrates. Here, the fabrication and characterization of OECTs with vertically stacked contacts, which overcome these limitations, is reported. The resulting vertical transistors exhibit a reduced footprint, increased intrinsic transconductance of up to 57 mS, and a geometry-normalized transconductance of 814 S m−1. The fabrication process is straightforward and compatible with sensitive organic materials, and allows exceptional control over the transistor channel length. This novel 3D fabrication method is particularly suited for applications where high density is needed, such as in implantable devices.
LanguageEnglish
Article number1705031
Number of pages5
JournalAdvanced Materials
Volume29
Early online date20 Dec 2017
DOIs
Publication statusE-pub ahead of print - 20 Dec 2017

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Transistors
Transconductance
Fabrication
Biocompatibility
Transducers
Availability
Geometry
Substrates

Keywords

  • electrochemical transistor
  • organic bioelectronics
  • transconductance
  • device density

Cite this

Donahue, M. J., Williamson, A., Strakosas, X., Friedlein, J. T., McLeod, R. R., Gleskova, H., & Malliaras, G. G. (2017). High performance vertical organic electrochemical transistors. Advanced Materials, 29, [1705031]. https://doi.org/10.1002/adma.201705031
Donahue, Mary J. ; Williamson, Adam ; Strakosas, Xenofon ; Friedlein, Jacob T. ; McLeod, Robert R. ; Gleskova, Helena ; Malliaras, George G. . / High performance vertical organic electrochemical transistors. In: Advanced Materials. 2017 ; Vol. 29.
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Donahue, MJ, Williamson, A, Strakosas, X, Friedlein, JT, McLeod, RR, Gleskova, H & Malliaras, GG 2017, 'High performance vertical organic electrochemical transistors' Advanced Materials, vol. 29, 1705031. https://doi.org/10.1002/adma.201705031

High performance vertical organic electrochemical transistors. / Donahue, Mary J. ; Williamson, Adam; Strakosas, Xenofon ; Friedlein, Jacob T. ; McLeod, Robert R. ; Gleskova, Helena; Malliaras, George G. .

In: Advanced Materials, Vol. 29, 1705031, 20.12.2017.

Research output: Contribution to journalArticle

TY - JOUR

T1 - High performance vertical organic electrochemical transistors

AU - Donahue, Mary J.

AU - Williamson, Adam

AU - Strakosas, Xenofon

AU - Friedlein, Jacob T.

AU - McLeod, Robert R.

AU - Gleskova, Helena

AU - Malliaras, George G.

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AB - Organic electrochemical transistors (OECTs) are promising transducers for biointerfacing due to their high transconductance, biocompatibility, and availability in a variety of form factors. Most OECTs reported to date, however, utilize rather large channels, limiting the transistor performance and resulting in a low transistor density. This is typically a consequence of limitations associated with traditional fabrication methods and with 2D substrates. Here, the fabrication and characterization of OECTs with vertically stacked contacts, which overcome these limitations, is reported. The resulting vertical transistors exhibit a reduced footprint, increased intrinsic transconductance of up to 57 mS, and a geometry-normalized transconductance of 814 S m−1. The fabrication process is straightforward and compatible with sensitive organic materials, and allows exceptional control over the transistor channel length. This novel 3D fabrication method is particularly suited for applications where high density is needed, such as in implantable devices.

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Donahue MJ, Williamson A, Strakosas X, Friedlein JT, McLeod RR, Gleskova H et al. High performance vertical organic electrochemical transistors. Advanced Materials. 2017 Dec 20;29. 1705031. https://doi.org/10.1002/adma.201705031