Heterodyne spectral interferometry for multidimensional nonlinear spectroscopy of individual quantum systems

Wolfgang Langbein; Brian Patton

doi:10.1364/OL.31.001151

Heterodyne spectral interferometry for multidimensional nonlinear spectroscopy of individual quantum systems

Wolfgang Langbein, Brian Patton

Physics

Research output: Contribution to journal › Article › peer-review

66 Citations (Scopus)

Abstract

A novel implementation of transient nonlinear spectroscopy is presented that allows the study of the transient nonlinear polarization emitted from individual electronic transitions. Both the amplitude and the phase of the polarization are retrieved, permitting the implementation of multidimensional spectroscopy in the excitation pulse delays. The technique is shown to detect mutual coherent coupling in a group of individual, localized excitonic transitions.

Original language	English
Pages (from-to)	1151-1153
Number of pages	3
Journal	Optics Letters
Volume	31
Issue number	8
DOIs	https://doi.org/10.1364/OL.31.001151
Publication status	Published - 20 Jan 2006

Keywords

nonlinear spectroscopy
transient nonlinear polarization
interference
phase shift

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10.1364/OL.31.001151

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title = "Heterodyne spectral interferometry for multidimensional nonlinear spectroscopy of individual quantum systems",

abstract = "A novel implementation of transient nonlinear spectroscopy is presented that allows the study of the transient nonlinear polarization emitted from individual electronic transitions. Both the amplitude and the phase of the polarization are retrieved, permitting the implementation of multidimensional spectroscopy in the excitation pulse delays. The technique is shown to detect mutual coherent coupling in a group of individual, localized excitonic transitions.",

keywords = "nonlinear spectroscopy, transient nonlinear polarization, interference, phase shift",

author = "Wolfgang Langbein and Brian Patton",

year = "2006",

month = jan,

day = "20",

doi = "10.1364/OL.31.001151",

language = "English",

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TY - JOUR

T1 - Heterodyne spectral interferometry for multidimensional nonlinear spectroscopy of individual quantum systems

AU - Langbein, Wolfgang

AU - Patton, Brian

PY - 2006/1/20

Y1 - 2006/1/20

N2 - A novel implementation of transient nonlinear spectroscopy is presented that allows the study of the transient nonlinear polarization emitted from individual electronic transitions. Both the amplitude and the phase of the polarization are retrieved, permitting the implementation of multidimensional spectroscopy in the excitation pulse delays. The technique is shown to detect mutual coherent coupling in a group of individual, localized excitonic transitions.

AB - A novel implementation of transient nonlinear spectroscopy is presented that allows the study of the transient nonlinear polarization emitted from individual electronic transitions. Both the amplitude and the phase of the polarization are retrieved, permitting the implementation of multidimensional spectroscopy in the excitation pulse delays. The technique is shown to detect mutual coherent coupling in a group of individual, localized excitonic transitions.

KW - nonlinear spectroscopy

KW - transient nonlinear polarization

KW - interference

KW - phase shift

U2 - 10.1364/OL.31.001151

DO - 10.1364/OL.31.001151

M3 - Article

SN - 0146-9592

VL - 31

SP - 1151

EP - 1153

JO - Optics Letters

JF - Optics Letters

IS - 8

ER -

Heterodyne spectral interferometry for multidimensional nonlinear spectroscopy of individual quantum systems

Abstract

Keywords

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