Evolution of the electrochemical interface in high-temperature fuel cells and electrolysers

John T.S. Irvine, Dragos Neagu, Maarten C. Verbraeken, Christodoulos Chatzichristodoulou, Christopher Graves, Mogens B. Mogensen

Research output: Contribution to journalReview article

240 Citations (Scopus)
3 Downloads (Pure)

Abstract

The critical region determining the performance and lifetime of solid oxide electrochemical systems is normally at the electrode side of the electrode/electrolyte interface. Typically this electrochemically active region only extends a few micrometres and for best performance involves intricate structures and nanocomposites. Much of the most exciting recent research involves understanding processes occurring at this interface and in developing new means of controlling the structure at this interface on the nanoscale. Here we consider in detail the diverse range of materials architectures that may be involved, describe the evolution of these interface structures and finally explore the new chemistries that allow control and manipulation of these architectures to optimize both performance and durability.

Original languageEnglish
Article number15014
JournalNature Energy
Volume1
Issue number1
DOIs
Publication statusPublished - 11 Jan 2016
Externally publishedYes

Keywords

  • solid oxide electrochemical systems
  • electrochemical electrodes
  • nanocomposites
  • fuel cells
  • electrolysers

Fingerprint Dive into the research topics of 'Evolution of the electrochemical interface in high-temperature fuel cells and electrolysers'. Together they form a unique fingerprint.

  • Cite this

    Irvine, J. T. S., Neagu, D., Verbraeken, M. C., Chatzichristodoulou, C., Graves, C., & Mogensen, M. B. (2016). Evolution of the electrochemical interface in high-temperature fuel cells and electrolysers. Nature Energy, 1(1), [15014]. https://doi.org/10.1038/nenergy.2015.14