This dataset contains a series of Bruker format frames in .sfrm format that can be read by APEX 2/3 software that were obtained for the characterisation of CO2/N2O binary crystal by single crystal X-ray diffraction. The Compressiondatasets.zip contains 5 datasets for the binary crystal on compression. Comp01 is at 2.0GPa, Comp02 at 2.3 Gpa; Comp03 at 2.6 GPa; Comp04 at 4 GPa; Comp06 5.2 GPa. Comp05 is not present due to an aborted run (power cut). The compound codes for the low temperature datasets are self explanatory composition appended with temperature at which the dataset was collected.